Performance evaluation of aqueous carbonation for steelmaking slag: Process chemistry

Shu Yuan Pan, Pen Chi Chiang, Yi Hung Chen, Chun Da Chen, Hsun Yu Lin, E. E. Chang

Research output: Contribution to journalArticle

4 Citations (Scopus)

Abstract

Accelerated carbonation of BOF slag in an RPB is a viable method for CO2 capture due to its high mass transfer rate. However, the process chemistry of carbonation of BOF slag is not well-determined due to their complex compositions. In this investigation, the quantitative X-ray diffraction was utilized to determine the mechanism of carbonation reaction in an RPB. Rietveld refinement, which aims to minimize the difference between the experimental and refined XRD patterns by a least-square procedure, is performed to quantify the crystallized mineral. In addition, changes of physico-chemical properties of BOF slags before and after carbonation were evaluated.

Original languageEnglish
Pages (from-to)115-121
Number of pages7
JournalEnergy Procedia
Volume37
DOIs
Publication statusPublished - 2013

Keywords

  • Calcite
  • CO sequestration
  • Quantitative X-ray diffraction; Rietveld method
  • Rotating packed bed
  • Thermogravimetric analysis

ASJC Scopus subject areas

  • Energy(all)

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  • Cite this

    Pan, S. Y., Chiang, P. C., Chen, Y. H., Chen, C. D., Lin, H. Y., & Chang, E. E. (2013). Performance evaluation of aqueous carbonation for steelmaking slag: Process chemistry. Energy Procedia, 37, 115-121. https://doi.org/10.1016/j.egypro.2013.05.091