Magnification of photonic crystal fluorescence enhancement via TM resonance excitation and TE resonance extraction on a dielectric nanorod surface

Hsin Yu Wu, Wei Zhang, Patrick C. Mathias, Brian T. Cunningham

Research output: Contribution to journalArticle

23 Citations (Scopus)

Abstract

Using a one-dimensional grating surface photonic crystal (PC), we experimentally demonstrate that the detection of fluorescent molecules on a PC surface can be substantially magnified through the combined effects of resonance-enhanced excitation of the fluorescent dye, resonance-enhanced extraction of the fluorescence emission and a dielectric nanorod surface coating increasing the surface area available for fluorophore-PC interaction. Enhanced excitation is obtained by engineering a high-Q TM resonant mode to efficiently couple with an incident TM-polarized λ = 633nm laser for exciting Cyanine-5 (Cy5). Enhanced extraction results from a low-Q TE resonance designed to spectrally overlap the Cy5 emission spectrum for channeling TE-polarized emission towards the detection instrument. The entire PC surface is coated with a porous film of TiO2 nanorods that allows more fluorophores to penetrate into the region of enhanced near-electric fields. Experimental results reveal a 588-fold enhancement in fluorescence intensity relative to an unpatterned glass surface.

Original languageEnglish
Article number125203
JournalNanotechnology
Volume21
Issue number12
DOIs
Publication statusPublished - 2010
Externally publishedYes

Fingerprint

Photonic crystals
Nanorods
Fluorescence
Fluorophores
Fluorescent Dyes
Dyes
Electric fields
Glass
Coatings
Molecules
Lasers

ASJC Scopus subject areas

  • Bioengineering
  • Chemistry(all)
  • Electrical and Electronic Engineering
  • Mechanical Engineering
  • Mechanics of Materials
  • Materials Science(all)

Cite this

Magnification of photonic crystal fluorescence enhancement via TM resonance excitation and TE resonance extraction on a dielectric nanorod surface. / Wu, Hsin Yu; Zhang, Wei; Mathias, Patrick C.; Cunningham, Brian T.

In: Nanotechnology, Vol. 21, No. 12, 125203, 2010.

Research output: Contribution to journalArticle

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